Uklanjanje uranil-jona iz rastvora kiselo tretiranim zeolitima
Removal of uranium (VI) from aqueous solution by acid modified zeolites

2016
Authors
Matijašević, SrđanZildžović, Snežana

Stojanović, Jovica

Đošić, Marija
Nikolić, Jelena
Stojanović, Mirjana
Labus, Nebojša

Article (Published version)
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Cilj ovog rada je prikaz mogućnosti primene prirodnog i modifikovanog zeolitskog minerala kao adsorbenta i materijala za sanaciju voda kontaminiranih uranijum jonom. Modifikovani uzorci zeolita dobijeni su tretiranjem prirodnog zeolita - klinoptilolita sa kiselinama: hlorovodoničnom, oksalnom i limunskom. Polazni i modifikovani zeoliti su okarakterisani hemijskom analizom, skenirajućom elektronskom mikroskopijom (SEM), rendgenskom analizom (XRPD), IC spektroskopijom, termičkom (TG/DTA) analizom i određivanjem kapaciteta katjonske izmene, a polazne i neadsorbovane količine uranijum jona su određene fluorimetrijski. Eksperimenti su sprovedeni da se ispita uticaj odnosa čvrsto/tečno, pH i vremena na adsorpciju uranijum jona na zeolitu. Utvrđeno je da tretman sa kiselinama zeolita povećava adsorpciju uranijum jona. Najviši indeks adsorpcije imao je uzorak zeolita modifikovan sa hlorovodoničnom kiselinom. Dobijeni rezultati adsorpcije na H-zeolitu su izračunati prema Langmirovom modelu.
...Projekat MPNTR, br. 142057
Razvoj stakala sa kontrolisanim otpuštanjem jona za primenu u poljoprivredi i medicini (MPNTR - 34001)
The objective of this study was the review of natural zeolite, modified with acid, as a candidate material for the remediation of groundwater contaminated by uranium(VI). The modified zeolite samples were obtained by treatment of natural zeolite - clinoptilolite with acids: hydrochloric, oxalyc and citric. Starting and modified zeolites were characterized by chemical analysis, SEM, XRPD analysis, IR spectroscopy, thermal (TG/DT) analysis and by determination of cation exchange capacity, while starting and nonadsorbed amounts of uranium(VI) ion were determined by fluorometric method. Batch experiments were conducted to investigate the effect of solid/liquid ratio, pH and time on the U(VI) uptake by zeolite. Modification of zeolitic tuff with acids significantly increased adsorption of uranium(VI). The highest adsorption of uranium(VI) ion was achieved on clinoptilolite modified with hydrochloric acid. Uranium(VI) adsorption data for zeolite modified with hydrochloric acid was fitted to ...the Langmuir model.
Projekat MPNTR, br. 142057
The development of glasses with controlled ions release for application in agriculture and medicine (MESTD - 34001)
Keywords:
zeolite-clinoptilolite / acid modification / uranium(VI) adsorptionSource:
Zaštita materijala, 2016, 57, 4, 551-558Funding / projects:
- The development of glasses with controlled ions release for application in agriculture and medicine (RS-34001)
- Fizičko-hemijski fenomeni površina alumosilikatnih minerala - osnova za razvoj novih ekoloških materijala (RS-142057)
Institution/Community
Институт техничких наука САНУ / Institute of Technical Sciences of SASATY - JOUR AU - Matijašević, Srđan AU - Zildžović, Snežana AU - Stojanović, Jovica AU - Đošić, Marija AU - Nikolić, Jelena AU - Stojanović, Mirjana AU - Labus, Nebojša PY - 2016 UR - https://dais.sanu.ac.rs/123456789/899 AB - Cilj ovog rada je prikaz mogućnosti primene prirodnog i modifikovanog zeolitskog minerala kao adsorbenta i materijala za sanaciju voda kontaminiranih uranijum jonom. Modifikovani uzorci zeolita dobijeni su tretiranjem prirodnog zeolita - klinoptilolita sa kiselinama: hlorovodoničnom, oksalnom i limunskom. Polazni i modifikovani zeoliti su okarakterisani hemijskom analizom, skenirajućom elektronskom mikroskopijom (SEM), rendgenskom analizom (XRPD), IC spektroskopijom, termičkom (TG/DTA) analizom i određivanjem kapaciteta katjonske izmene, a polazne i neadsorbovane količine uranijum jona su određene fluorimetrijski. Eksperimenti su sprovedeni da se ispita uticaj odnosa čvrsto/tečno, pH i vremena na adsorpciju uranijum jona na zeolitu. Utvrđeno je da tretman sa kiselinama zeolita povećava adsorpciju uranijum jona. Najviši indeks adsorpcije imao je uzorak zeolita modifikovan sa hlorovodoničnom kiselinom. Dobijeni rezultati adsorpcije na H-zeolitu su izračunati prema Langmirovom modelu. Projekat MPNTR, br. 142057 Razvoj stakala sa kontrolisanim otpuštanjem jona za primenu u poljoprivredi i medicini (MPNTR - 34001) AB - The objective of this study was the review of natural zeolite, modified with acid, as a candidate material for the remediation of groundwater contaminated by uranium(VI). The modified zeolite samples were obtained by treatment of natural zeolite - clinoptilolite with acids: hydrochloric, oxalyc and citric. Starting and modified zeolites were characterized by chemical analysis, SEM, XRPD analysis, IR spectroscopy, thermal (TG/DT) analysis and by determination of cation exchange capacity, while starting and nonadsorbed amounts of uranium(VI) ion were determined by fluorometric method. Batch experiments were conducted to investigate the effect of solid/liquid ratio, pH and time on the U(VI) uptake by zeolite. Modification of zeolitic tuff with acids significantly increased adsorption of uranium(VI). The highest adsorption of uranium(VI) ion was achieved on clinoptilolite modified with hydrochloric acid. Uranium(VI) adsorption data for zeolite modified with hydrochloric acid was fitted to the Langmuir model. Projekat MPNTR, br. 142057 The development of glasses with controlled ions release for application in agriculture and medicine (MESTD - 34001) T2 - Zaštita materijala T1 - Uklanjanje uranil-jona iz rastvora kiselo tretiranim zeolitima SP - 551 EP - 558 VL - 57 IS - 4 DO - 10.5937/ZasMat1604551M UR - https://hdl.handle.net/21.15107/rcub_dais_899 ER -
@article{ author = "Matijašević, Srđan and Zildžović, Snežana and Stojanović, Jovica and Đošić, Marija and Nikolić, Jelena and Stojanović, Mirjana and Labus, Nebojša", year = "2016", abstract = "Cilj ovog rada je prikaz mogućnosti primene prirodnog i modifikovanog zeolitskog minerala kao adsorbenta i materijala za sanaciju voda kontaminiranih uranijum jonom. Modifikovani uzorci zeolita dobijeni su tretiranjem prirodnog zeolita - klinoptilolita sa kiselinama: hlorovodoničnom, oksalnom i limunskom. Polazni i modifikovani zeoliti su okarakterisani hemijskom analizom, skenirajućom elektronskom mikroskopijom (SEM), rendgenskom analizom (XRPD), IC spektroskopijom, termičkom (TG/DTA) analizom i određivanjem kapaciteta katjonske izmene, a polazne i neadsorbovane količine uranijum jona su određene fluorimetrijski. Eksperimenti su sprovedeni da se ispita uticaj odnosa čvrsto/tečno, pH i vremena na adsorpciju uranijum jona na zeolitu. Utvrđeno je da tretman sa kiselinama zeolita povećava adsorpciju uranijum jona. Najviši indeks adsorpcije imao je uzorak zeolita modifikovan sa hlorovodoničnom kiselinom. Dobijeni rezultati adsorpcije na H-zeolitu su izračunati prema Langmirovom modelu. Projekat MPNTR, br. 142057 Razvoj stakala sa kontrolisanim otpuštanjem jona za primenu u poljoprivredi i medicini (MPNTR - 34001), The objective of this study was the review of natural zeolite, modified with acid, as a candidate material for the remediation of groundwater contaminated by uranium(VI). The modified zeolite samples were obtained by treatment of natural zeolite - clinoptilolite with acids: hydrochloric, oxalyc and citric. Starting and modified zeolites were characterized by chemical analysis, SEM, XRPD analysis, IR spectroscopy, thermal (TG/DT) analysis and by determination of cation exchange capacity, while starting and nonadsorbed amounts of uranium(VI) ion were determined by fluorometric method. Batch experiments were conducted to investigate the effect of solid/liquid ratio, pH and time on the U(VI) uptake by zeolite. Modification of zeolitic tuff with acids significantly increased adsorption of uranium(VI). The highest adsorption of uranium(VI) ion was achieved on clinoptilolite modified with hydrochloric acid. Uranium(VI) adsorption data for zeolite modified with hydrochloric acid was fitted to the Langmuir model. Projekat MPNTR, br. 142057 The development of glasses with controlled ions release for application in agriculture and medicine (MESTD - 34001)", journal = "Zaštita materijala", title = "Uklanjanje uranil-jona iz rastvora kiselo tretiranim zeolitima", pages = "551-558", volume = "57", number = "4", doi = "10.5937/ZasMat1604551M", url = "https://hdl.handle.net/21.15107/rcub_dais_899" }
Matijašević, S., Zildžović, S., Stojanović, J., Đošić, M., Nikolić, J., Stojanović, M.,& Labus, N.. (2016). Uklanjanje uranil-jona iz rastvora kiselo tretiranim zeolitima. in Zaštita materijala, 57(4), 551-558. https://doi.org/10.5937/ZasMat1604551M https://hdl.handle.net/21.15107/rcub_dais_899
Matijašević S, Zildžović S, Stojanović J, Đošić M, Nikolić J, Stojanović M, Labus N. Uklanjanje uranil-jona iz rastvora kiselo tretiranim zeolitima. in Zaštita materijala. 2016;57(4):551-558. doi:10.5937/ZasMat1604551M https://hdl.handle.net/21.15107/rcub_dais_899 .
Matijašević, Srđan, Zildžović, Snežana, Stojanović, Jovica, Đošić, Marija, Nikolić, Jelena, Stojanović, Mirjana, Labus, Nebojša, "Uklanjanje uranil-jona iz rastvora kiselo tretiranim zeolitima" in Zaštita materijala, 57, no. 4 (2016):551-558, https://doi.org/10.5937/ZasMat1604551M ., https://hdl.handle.net/21.15107/rcub_dais_899 .