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Kinetics of hydrogen absorption in Zr-based alloys

Authorized Users Only
2013
Authors
Cekić, Božidar
Ćirić, Katarina
Iordoc, Mihail
Marković, Smilja
Mitrić, Miodrag
Article (Published version)
Metadata
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Abstract
The kinetics of hydrogen absorption in Zr-based alloys Zr–2.5Nb, Zr–10Nb, Zr–2.5Nb–3Ta and Zr–10Nb–12Ta have been investigated in the temperature range 673–973 K at 1 bar hydrogen pressure. The improvement in hydrogen kinetics and a slight decrease of maximal amount of hydrogen absorbed were observed upon cycling. The rate determining steps are as follows: geometrical contraction for all samples except Zr–10Nb–12Ta; diffusion in the beginning for Zr–10Nb at 973 K Zr–2.5Nb–3Ta at 673 K and 973 K; first order reaction Zr–10Nb–12Ta at all temperatures. The amount of additives, Nb and Ta, is found to have major influence on the mechanism of the absorption process.
Keywords:
hydrogen absorbing materials / zirconium alloys / kinetics / hydriding isotherm
Source:
Journal of Alloys and Compounds, 2013, 559, 162-166
Publisher:
  • Elsevier
Funding / projects:
  • Nanostructured multifunctional materials and nanocomposites (RS-45018)

DOI: 10.1016/j.jallcom.2013.01.104

ISSN: 0925-8388

WoS: 000316679800029

Scopus: 2-s2.0-84874094886
[ Google Scholar ]
18
11
Handle
https://hdl.handle.net/21.15107/rcub_dais_342
URI
https://dais.sanu.ac.rs/123456789/342
Collections
  • ИТН САНУ - Општа колекција / ITS SASA - General collection
Institution/Community
Институт техничких наука САНУ / Institute of Technical Sciences of SASA
TY  - JOUR
AU  - Cekić, Božidar
AU  - Ćirić, Katarina
AU  - Iordoc, Mihail
AU  - Marković, Smilja
AU  - Mitrić, Miodrag
PY  - 2013
UR  - https://dais.sanu.ac.rs/123456789/342
AB  - The kinetics of hydrogen absorption in Zr-based alloys Zr–2.5Nb, Zr–10Nb, Zr–2.5Nb–3Ta and Zr–10Nb–12Ta have been investigated in the temperature range 673–973 K at 1 bar hydrogen pressure. The improvement in hydrogen kinetics and a slight decrease of maximal amount of hydrogen absorbed were observed upon cycling. The rate determining steps are as follows: geometrical contraction for all samples except Zr–10Nb–12Ta; diffusion in the beginning for Zr–10Nb at 973 K Zr–2.5Nb–3Ta at 673 K and 973 K; first order reaction Zr–10Nb–12Ta at all temperatures. The amount of additives, Nb and Ta, is found to have major influence on the mechanism of the absorption process.
PB  - Elsevier
T2  - Journal of Alloys and Compounds
T1  - Kinetics of hydrogen absorption in Zr-based alloys
SP  - 162
EP  - 166
VL  - 559
DO  - 10.1016/j.jallcom.2013.01.104
UR  - https://hdl.handle.net/21.15107/rcub_dais_342
ER  - 
@article{
author = "Cekić, Božidar and Ćirić, Katarina and Iordoc, Mihail and Marković, Smilja and Mitrić, Miodrag",
year = "2013",
abstract = "The kinetics of hydrogen absorption in Zr-based alloys Zr–2.5Nb, Zr–10Nb, Zr–2.5Nb–3Ta and Zr–10Nb–12Ta have been investigated in the temperature range 673–973 K at 1 bar hydrogen pressure. The improvement in hydrogen kinetics and a slight decrease of maximal amount of hydrogen absorbed were observed upon cycling. The rate determining steps are as follows: geometrical contraction for all samples except Zr–10Nb–12Ta; diffusion in the beginning for Zr–10Nb at 973 K Zr–2.5Nb–3Ta at 673 K and 973 K; first order reaction Zr–10Nb–12Ta at all temperatures. The amount of additives, Nb and Ta, is found to have major influence on the mechanism of the absorption process.",
publisher = "Elsevier",
journal = "Journal of Alloys and Compounds",
title = "Kinetics of hydrogen absorption in Zr-based alloys",
pages = "162-166",
volume = "559",
doi = "10.1016/j.jallcom.2013.01.104",
url = "https://hdl.handle.net/21.15107/rcub_dais_342"
}
Cekić, B., Ćirić, K., Iordoc, M., Marković, S.,& Mitrić, M.. (2013). Kinetics of hydrogen absorption in Zr-based alloys. in Journal of Alloys and Compounds
Elsevier., 559, 162-166.
https://doi.org/10.1016/j.jallcom.2013.01.104
https://hdl.handle.net/21.15107/rcub_dais_342
Cekić B, Ćirić K, Iordoc M, Marković S, Mitrić M. Kinetics of hydrogen absorption in Zr-based alloys. in Journal of Alloys and Compounds. 2013;559:162-166.
doi:10.1016/j.jallcom.2013.01.104
https://hdl.handle.net/21.15107/rcub_dais_342 .
Cekić, Božidar, Ćirić, Katarina, Iordoc, Mihail, Marković, Smilja, Mitrić, Miodrag, "Kinetics of hydrogen absorption in Zr-based alloys" in Journal of Alloys and Compounds, 559 (2013):162-166,
https://doi.org/10.1016/j.jallcom.2013.01.104 .,
https://hdl.handle.net/21.15107/rcub_dais_342 .

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