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Structural and functional properties of ZnO thin films grown on Si substrates by air assisted USP method from non-aqueous solutions at low-temperature

Authorized Users Only
2017
Authors
Flores-Carrasco, Gregorio
Muñoz-Fernandez, Lidia
Alcántara-Iniesta, Salvador
Soto-Cruz, Blanca Susana
Milošević, Olivera
Rabanal, Maria Eugenia
Article (Published version)
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Abstract
In this work, we deals with the processing and characterization of transparent conducting ZnO thin films on p-type Silicon substrates (1 0 0) by air assisted Ultrasonic Spray Pyrolysis (USP) method. The thin films from different Zn acetate precursor solution concentrations (0.1, 0.2, 0.3 and 0.4 M) were deposited at several temperatures (400, 450 and 500 °C) with thickness from ∼100 to ∼500 nm. The effects of precursor solution concentration, deposition time and temperature on the structural, morphological, optical, and electrical properties of ZnO films were studied by X-ray Diffraction (XRD), Atomic Force Microscopy (AFM), UV–Vis-NIR spectroscopy, and Hall Effect techniques, respectively. It has been shown that on the ZnO film surface, the preferred orientation, the average crystallite size, the electrical resistivity and the RMS surface roughness depend on the substrate temperature. The grown films have showed a good adhesion and an excellent optical transmission of about 80–95% wit...hin the visible range (400–800 nm) and a direct band gap from 3.35 to 3.23 eV with the increase of the substrate temperature and the deposition time. All the PL spectra have exhibited a typical green-yellow emission band. Additionally photovoltaic (PV) activities of n-ZnO/p-Si heterostructures fabricated are investigated.

Keywords:
n-ZnO/p-Si / Ultrasonic spray pyrolysis / Electro-optical properties
Source:
Advanced Powder Technology, 2017, 28, 1, 93-100
Funding / projects:
  • Materials of Reduced Dimensions for Efficient Light Harvesting and Energy conversion (RS-45020)

DOI: 10.1016/j.apt.2016.11.016

ISSN: 0921-8831

WoS: 000395355100012

Scopus: 2-s2.0-85008403658
[ Google Scholar ]
5
5
Handle
https://hdl.handle.net/21.15107/rcub_dais_15458
URI
https://dais.sanu.ac.rs/123456789/15458
Collections
  • ИТН САНУ - Општа колекција / ITS SASA - General collection
Institution/Community
Институт техничких наука САНУ / Institute of Technical Sciences of SASA
TY  - JOUR
AU  - Flores-Carrasco, Gregorio
AU  - Muñoz-Fernandez, Lidia
AU  - Alcántara-Iniesta, Salvador
AU  - Soto-Cruz, Blanca Susana
AU  - Milošević, Olivera
AU  - Rabanal, Maria Eugenia
PY  - 2017
UR  - https://dais.sanu.ac.rs/123456789/15458
AB  - In this work, we deals with the processing and characterization of transparent conducting ZnO thin films on p-type Silicon substrates (1 0 0) by air assisted Ultrasonic Spray Pyrolysis (USP) method. The thin films from different Zn acetate precursor solution concentrations (0.1, 0.2, 0.3 and 0.4 M) were deposited at several temperatures (400, 450 and 500 °C) with thickness from ∼100 to ∼500 nm. The effects of precursor solution concentration, deposition time and temperature on the structural, morphological, optical, and electrical properties of ZnO films were studied by X-ray Diffraction (XRD), Atomic Force Microscopy (AFM), UV–Vis-NIR spectroscopy, and Hall Effect techniques, respectively. It has been shown that on the ZnO film surface, the preferred orientation, the average crystallite size, the electrical resistivity and the RMS surface roughness depend on the substrate temperature. The grown films have showed a good adhesion and an excellent optical transmission of about 80–95% within the visible range (400–800 nm) and a direct band gap from 3.35 to 3.23 eV with the increase of the substrate temperature and the deposition time. All the PL spectra have exhibited a typical green-yellow emission band. Additionally photovoltaic (PV) activities of n-ZnO/p-Si heterostructures fabricated are investigated.
T2  - Advanced Powder Technology
T1  - Structural and functional properties of ZnO thin films grown on Si substrates by air assisted USP method from non-aqueous solutions at low-temperature
SP  - 93
EP  - 100
VL  - 28
IS  - 1
DO  - 10.1016/j.apt.2016.11.016
UR  - https://hdl.handle.net/21.15107/rcub_dais_15458
ER  - 
@article{
author = "Flores-Carrasco, Gregorio and Muñoz-Fernandez, Lidia and Alcántara-Iniesta, Salvador and Soto-Cruz, Blanca Susana and Milošević, Olivera and Rabanal, Maria Eugenia",
year = "2017",
abstract = "In this work, we deals with the processing and characterization of transparent conducting ZnO thin films on p-type Silicon substrates (1 0 0) by air assisted Ultrasonic Spray Pyrolysis (USP) method. The thin films from different Zn acetate precursor solution concentrations (0.1, 0.2, 0.3 and 0.4 M) were deposited at several temperatures (400, 450 and 500 °C) with thickness from ∼100 to ∼500 nm. The effects of precursor solution concentration, deposition time and temperature on the structural, morphological, optical, and electrical properties of ZnO films were studied by X-ray Diffraction (XRD), Atomic Force Microscopy (AFM), UV–Vis-NIR spectroscopy, and Hall Effect techniques, respectively. It has been shown that on the ZnO film surface, the preferred orientation, the average crystallite size, the electrical resistivity and the RMS surface roughness depend on the substrate temperature. The grown films have showed a good adhesion and an excellent optical transmission of about 80–95% within the visible range (400–800 nm) and a direct band gap from 3.35 to 3.23 eV with the increase of the substrate temperature and the deposition time. All the PL spectra have exhibited a typical green-yellow emission band. Additionally photovoltaic (PV) activities of n-ZnO/p-Si heterostructures fabricated are investigated.",
journal = "Advanced Powder Technology",
title = "Structural and functional properties of ZnO thin films grown on Si substrates by air assisted USP method from non-aqueous solutions at low-temperature",
pages = "93-100",
volume = "28",
number = "1",
doi = "10.1016/j.apt.2016.11.016",
url = "https://hdl.handle.net/21.15107/rcub_dais_15458"
}
Flores-Carrasco, G., Muñoz-Fernandez, L., Alcántara-Iniesta, S., Soto-Cruz, B. S., Milošević, O.,& Rabanal, M. E.. (2017). Structural and functional properties of ZnO thin films grown on Si substrates by air assisted USP method from non-aqueous solutions at low-temperature. in Advanced Powder Technology, 28(1), 93-100.
https://doi.org/10.1016/j.apt.2016.11.016
https://hdl.handle.net/21.15107/rcub_dais_15458
Flores-Carrasco G, Muñoz-Fernandez L, Alcántara-Iniesta S, Soto-Cruz BS, Milošević O, Rabanal ME. Structural and functional properties of ZnO thin films grown on Si substrates by air assisted USP method from non-aqueous solutions at low-temperature. in Advanced Powder Technology. 2017;28(1):93-100.
doi:10.1016/j.apt.2016.11.016
https://hdl.handle.net/21.15107/rcub_dais_15458 .
Flores-Carrasco, Gregorio, Muñoz-Fernandez, Lidia, Alcántara-Iniesta, Salvador, Soto-Cruz, Blanca Susana, Milošević, Olivera, Rabanal, Maria Eugenia, "Structural and functional properties of ZnO thin films grown on Si substrates by air assisted USP method from non-aqueous solutions at low-temperature" in Advanced Powder Technology, 28, no. 1 (2017):93-100,
https://doi.org/10.1016/j.apt.2016.11.016 .,
https://hdl.handle.net/21.15107/rcub_dais_15458 .

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