Bamboo‐Membrane Inspired Multilevel Ultrafast Interlayer Ion Transport for Superior Volumetric Energy Storage
Abstract
Interlayer transport of charges and carriers of 2D nanomaterials is a critical parameter that governs the material and device performance in energy storage applications. Inspired by multilevel natural bamboo-membrane with ultrafast water and electrolyte transport properties to support its super-rapid growth rate, 2D–2D multilevel heterostructured graphene-based membranes with tailored gradient interlayer channels are rationally designed for achieving ultrafast interlayer ion transport. The bioinspired heterostructured membranes possess multilevel interlayer spacing distributions, where the closely packed layers with sub-nanosized interlayer space provide ultrafast confined interlayer ion transport, while the loosely stacked outer layers consisting of open channels with large distances up to few micrometres are favorable for rapid wetting and penetration of liquid electrolytes. The combination of advantages of large-size open channels and nanosized confined channels offers ultrafast ele...ctrolyte wetting and permeation and interlayer ion transport and provide the devices with superior volumetric capacity as free-standing electrodes for rechargeable batteries.
Keywords:
nanomaterials / interlayer transport / energy storageSource:
Advanced Functional Materials, 2021, 31, 31, 2100299-Publisher:
- Wiley
Funding / projects:
- National Natural Science Foundation of China: 51671085
- https://doi.org/10.13039/501100001809
DOI: 10.1002/adfm.202100299
ISSN: 1616-301X; 1616-3028
WoS: 000653209900001
Scopus: 2-s2.0-85106337861
Institution/Community
Институт техничких наука САНУ / Institute of Technical Sciences of SASATY - JOUR AU - Mei, Jun AU - Peng, Xiaomin AU - Zhang, Qian AU - Zhang, Xiaoqi AU - Liao, Ting AU - Mitić, Vojislav V. AU - Sun, Ziqi PY - 2021 UR - https://dais.sanu.ac.rs/123456789/11801 AB - Interlayer transport of charges and carriers of 2D nanomaterials is a critical parameter that governs the material and device performance in energy storage applications. Inspired by multilevel natural bamboo-membrane with ultrafast water and electrolyte transport properties to support its super-rapid growth rate, 2D–2D multilevel heterostructured graphene-based membranes with tailored gradient interlayer channels are rationally designed for achieving ultrafast interlayer ion transport. The bioinspired heterostructured membranes possess multilevel interlayer spacing distributions, where the closely packed layers with sub-nanosized interlayer space provide ultrafast confined interlayer ion transport, while the loosely stacked outer layers consisting of open channels with large distances up to few micrometres are favorable for rapid wetting and penetration of liquid electrolytes. The combination of advantages of large-size open channels and nanosized confined channels offers ultrafast electrolyte wetting and permeation and interlayer ion transport and provide the devices with superior volumetric capacity as free-standing electrodes for rechargeable batteries. PB - Wiley T2 - Advanced Functional Materials T1 - Bamboo‐Membrane Inspired Multilevel Ultrafast Interlayer Ion Transport for Superior Volumetric Energy Storage SP - 2100299 VL - 31 IS - 31 DO - 10.1002/adfm.202100299 UR - https://hdl.handle.net/21.15107/rcub_dais_11801 ER -
@article{ author = "Mei, Jun and Peng, Xiaomin and Zhang, Qian and Zhang, Xiaoqi and Liao, Ting and Mitić, Vojislav V. and Sun, Ziqi", year = "2021", abstract = "Interlayer transport of charges and carriers of 2D nanomaterials is a critical parameter that governs the material and device performance in energy storage applications. Inspired by multilevel natural bamboo-membrane with ultrafast water and electrolyte transport properties to support its super-rapid growth rate, 2D–2D multilevel heterostructured graphene-based membranes with tailored gradient interlayer channels are rationally designed for achieving ultrafast interlayer ion transport. The bioinspired heterostructured membranes possess multilevel interlayer spacing distributions, where the closely packed layers with sub-nanosized interlayer space provide ultrafast confined interlayer ion transport, while the loosely stacked outer layers consisting of open channels with large distances up to few micrometres are favorable for rapid wetting and penetration of liquid electrolytes. The combination of advantages of large-size open channels and nanosized confined channels offers ultrafast electrolyte wetting and permeation and interlayer ion transport and provide the devices with superior volumetric capacity as free-standing electrodes for rechargeable batteries.", publisher = "Wiley", journal = "Advanced Functional Materials", title = "Bamboo‐Membrane Inspired Multilevel Ultrafast Interlayer Ion Transport for Superior Volumetric Energy Storage", pages = "2100299", volume = "31", number = "31", doi = "10.1002/adfm.202100299", url = "https://hdl.handle.net/21.15107/rcub_dais_11801" }
Mei, J., Peng, X., Zhang, Q., Zhang, X., Liao, T., Mitić, V. V.,& Sun, Z.. (2021). Bamboo‐Membrane Inspired Multilevel Ultrafast Interlayer Ion Transport for Superior Volumetric Energy Storage. in Advanced Functional Materials Wiley., 31(31), 2100299. https://doi.org/10.1002/adfm.202100299 https://hdl.handle.net/21.15107/rcub_dais_11801
Mei J, Peng X, Zhang Q, Zhang X, Liao T, Mitić VV, Sun Z. Bamboo‐Membrane Inspired Multilevel Ultrafast Interlayer Ion Transport for Superior Volumetric Energy Storage. in Advanced Functional Materials. 2021;31(31):2100299. doi:10.1002/adfm.202100299 https://hdl.handle.net/21.15107/rcub_dais_11801 .
Mei, Jun, Peng, Xiaomin, Zhang, Qian, Zhang, Xiaoqi, Liao, Ting, Mitić, Vojislav V., Sun, Ziqi, "Bamboo‐Membrane Inspired Multilevel Ultrafast Interlayer Ion Transport for Superior Volumetric Energy Storage" in Advanced Functional Materials, 31, no. 31 (2021):2100299, https://doi.org/10.1002/adfm.202100299 ., https://hdl.handle.net/21.15107/rcub_dais_11801 .