Horváth, Endre

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  • Horváth, Endre (4)
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Author's Bibliography

Photocatalytic activity of N-TiO2 nanotubes decorated with CdS QD

Vujančević, Jelena; Bjelajac, Anđelika; Horváth, Endre; Forró, Laszlo; Pavlović, Vladimir B.; Janaćković, Đorđe

(Belgrade : Materials Research Society of Serbia, 2022)

TY  - CONF
AU  - Vujančević, Jelena
AU  - Bjelajac, Anđelika
AU  - Horváth, Endre
AU  - Forró, Laszlo
AU  - Pavlović, Vladimir B.
AU  - Janaćković, Đorđe
PY  - 2022
UR  - https://dais.sanu.ac.rs/123456789/13597
AB  - The negative consequences of the modern world are environmental pollution. To decrease it, a lot of research is focused on finding solution for its remediation. Photoactive materials have ability to utilize solar energy for the degradation of organic and inorganic pollutants. Among different photoactive material TiO2 has advantages due to its non-toxicity, chemical stability and corrosion resistance. The aim of this study was to investigate the synergetic effect of nitrogen incorporation into crystal structure of TiO2 and deposition of CdS onto amelioration of the photocatalytic degradation of methylen orange compared to the pristine TiO2. For that purpose TiO2 nanotubes were obtained by anodization of titanium foil in HF containing electrolyte. To achieve crystal structure and at the same time to introduce nitrogen in TiO2, the samples were annealed in ammonia atmosphere at 450 °C, for different time of annealing. The highest amount of nitrogen was achieved for the shortest time of annealing (30 min). Beside that, it was observed that the highest level of interstitial nitrogen was also achieved for the shortest time of annealing. Further, CdS quantum dots (QDs) were deposited on the nitrogen doped TiO2 nanotubes via an ex-situ method (using binding reagent). According to the FESEM micrographs, a partial agglomeration of CdS QDs on some domaines on top of the nanotubes was observed. By performing the DRS, the improvement of the optical response after nitrogen doping and deposition of CdS was demonstrated. The sample with the highest amount of total nitrogen and interstitial nitrogen in combination with deposition CdS QDs exhibited the highest photocatalytic efficiency.
PB  - Belgrade : Materials Research Society of Serbia
C3  - Program and The Book of abstracts / Twenty-third Annual Conference YUCOMAT 2022 & Twelfth World Round Table Conference on Sintering XII WRTCS 2022, Herceg Novi, Montenegro, August 29 - September 2, 2022
T1  - Photocatalytic activity of N-TiO2 nanotubes decorated with CdS QD
SP  - 140
EP  - 140
UR  - https://hdl.handle.net/21.15107/rcub_dais_13597
ER  - 
@conference{
author = "Vujančević, Jelena and Bjelajac, Anđelika and Horváth, Endre and Forró, Laszlo and Pavlović, Vladimir B. and Janaćković, Đorđe",
year = "2022",
abstract = "The negative consequences of the modern world are environmental pollution. To decrease it, a lot of research is focused on finding solution for its remediation. Photoactive materials have ability to utilize solar energy for the degradation of organic and inorganic pollutants. Among different photoactive material TiO2 has advantages due to its non-toxicity, chemical stability and corrosion resistance. The aim of this study was to investigate the synergetic effect of nitrogen incorporation into crystal structure of TiO2 and deposition of CdS onto amelioration of the photocatalytic degradation of methylen orange compared to the pristine TiO2. For that purpose TiO2 nanotubes were obtained by anodization of titanium foil in HF containing electrolyte. To achieve crystal structure and at the same time to introduce nitrogen in TiO2, the samples were annealed in ammonia atmosphere at 450 °C, for different time of annealing. The highest amount of nitrogen was achieved for the shortest time of annealing (30 min). Beside that, it was observed that the highest level of interstitial nitrogen was also achieved for the shortest time of annealing. Further, CdS quantum dots (QDs) were deposited on the nitrogen doped TiO2 nanotubes via an ex-situ method (using binding reagent). According to the FESEM micrographs, a partial agglomeration of CdS QDs on some domaines on top of the nanotubes was observed. By performing the DRS, the improvement of the optical response after nitrogen doping and deposition of CdS was demonstrated. The sample with the highest amount of total nitrogen and interstitial nitrogen in combination with deposition CdS QDs exhibited the highest photocatalytic efficiency.",
publisher = "Belgrade : Materials Research Society of Serbia",
journal = "Program and The Book of abstracts / Twenty-third Annual Conference YUCOMAT 2022 & Twelfth World Round Table Conference on Sintering XII WRTCS 2022, Herceg Novi, Montenegro, August 29 - September 2, 2022",
title = "Photocatalytic activity of N-TiO2 nanotubes decorated with CdS QD",
pages = "140-140",
url = "https://hdl.handle.net/21.15107/rcub_dais_13597"
}
Vujančević, J., Bjelajac, A., Horváth, E., Forró, L., Pavlović, V. B.,& Janaćković, Đ.. (2022). Photocatalytic activity of N-TiO2 nanotubes decorated with CdS QD. in Program and The Book of abstracts / Twenty-third Annual Conference YUCOMAT 2022 & Twelfth World Round Table Conference on Sintering XII WRTCS 2022, Herceg Novi, Montenegro, August 29 - September 2, 2022
Belgrade : Materials Research Society of Serbia., 140-140.
https://hdl.handle.net/21.15107/rcub_dais_13597
Vujančević J, Bjelajac A, Horváth E, Forró L, Pavlović VB, Janaćković Đ. Photocatalytic activity of N-TiO2 nanotubes decorated with CdS QD. in Program and The Book of abstracts / Twenty-third Annual Conference YUCOMAT 2022 & Twelfth World Round Table Conference on Sintering XII WRTCS 2022, Herceg Novi, Montenegro, August 29 - September 2, 2022. 2022;:140-140.
https://hdl.handle.net/21.15107/rcub_dais_13597 .
Vujančević, Jelena, Bjelajac, Anđelika, Horváth, Endre, Forró, Laszlo, Pavlović, Vladimir B., Janaćković, Đorđe, "Photocatalytic activity of N-TiO2 nanotubes decorated with CdS QD" in Program and The Book of abstracts / Twenty-third Annual Conference YUCOMAT 2022 & Twelfth World Round Table Conference on Sintering XII WRTCS 2022, Herceg Novi, Montenegro, August 29 - September 2, 2022 (2022):140-140,
https://hdl.handle.net/21.15107/rcub_dais_13597 .

Characteristic of photodiode based on vanadium oxide-TiO2 nanotubes/CH3NH3PbI3

Vujančević, Jelena; Blagojević, Vladimir A.; Andričević, Pavao; Pavlović, Vera P.; Horváth, Endre; Forró, László; Vlahović, Branislav; Pavlović, Vladimir B.; Janaćković, Đorđe

(Belgrade : Serbian Ceramic Society, 2022)

TY  - CONF
AU  - Vujančević, Jelena
AU  - Blagojević, Vladimir A.
AU  - Andričević, Pavao
AU  - Pavlović, Vera P.
AU  - Horváth, Endre
AU  - Forró, László
AU  - Vlahović, Branislav
AU  - Pavlović, Vladimir B.
AU  - Janaćković, Đorđe
PY  - 2022
UR  - https://dais.sanu.ac.rs/123456789/13627
AB  - The aim of this study was to investigate the influence of the deposition of vanadium oxide epitaxial layer on the photoresponse of TiO2/CH3NH3PbI3 heterojunction. TiO2 nanotube array was synthesized via anodization of titanium foil at three different voltages. After annealing at 450 °C, vanadium oxide was deposited by direct deposition from vanadyl(IV) sulfate solution. Microstructure analysis has been used for the investigation of the influence of different voltages of anodization on tube diameter. Spectroscopy measurements pointed out the red shift in diffusion reflectance spectra after deposition of vanadium oxide. The presence of V5+ oxidation state has been detected on the surface of nanotube arrays by chemical analysis. CH3NH3PbI3 monocrystal was dry pressed on top of the nanotubes in order to make a photodiode. The current-voltage characteristics of the photodiode were recorded and it was observed that the sample with the smallest wall thickness and higher amount of vanadium has the best photocurrent response.
PB  - Belgrade : Serbian Ceramic Society
C3  - Program and the Book of abstracts / Serbian Ceramic Society Conference Advanced Ceramics and Application X New Frontiers in Multifunctional Material Science and Processing, Serbia, Belgrade, 26-27. September 2022.
T1  - Characteristic of photodiode based on vanadium oxide-TiO2 nanotubes/CH3NH3PbI3
SP  - 90
EP  - 90
UR  - https://hdl.handle.net/21.15107/rcub_dais_13627
ER  - 
@conference{
author = "Vujančević, Jelena and Blagojević, Vladimir A. and Andričević, Pavao and Pavlović, Vera P. and Horváth, Endre and Forró, László and Vlahović, Branislav and Pavlović, Vladimir B. and Janaćković, Đorđe",
year = "2022",
abstract = "The aim of this study was to investigate the influence of the deposition of vanadium oxide epitaxial layer on the photoresponse of TiO2/CH3NH3PbI3 heterojunction. TiO2 nanotube array was synthesized via anodization of titanium foil at three different voltages. After annealing at 450 °C, vanadium oxide was deposited by direct deposition from vanadyl(IV) sulfate solution. Microstructure analysis has been used for the investigation of the influence of different voltages of anodization on tube diameter. Spectroscopy measurements pointed out the red shift in diffusion reflectance spectra after deposition of vanadium oxide. The presence of V5+ oxidation state has been detected on the surface of nanotube arrays by chemical analysis. CH3NH3PbI3 monocrystal was dry pressed on top of the nanotubes in order to make a photodiode. The current-voltage characteristics of the photodiode were recorded and it was observed that the sample with the smallest wall thickness and higher amount of vanadium has the best photocurrent response.",
publisher = "Belgrade : Serbian Ceramic Society",
journal = "Program and the Book of abstracts / Serbian Ceramic Society Conference Advanced Ceramics and Application X New Frontiers in Multifunctional Material Science and Processing, Serbia, Belgrade, 26-27. September 2022.",
title = "Characteristic of photodiode based on vanadium oxide-TiO2 nanotubes/CH3NH3PbI3",
pages = "90-90",
url = "https://hdl.handle.net/21.15107/rcub_dais_13627"
}
Vujančević, J., Blagojević, V. A., Andričević, P., Pavlović, V. P., Horváth, E., Forró, L., Vlahović, B., Pavlović, V. B.,& Janaćković, Đ.. (2022). Characteristic of photodiode based on vanadium oxide-TiO2 nanotubes/CH3NH3PbI3. in Program and the Book of abstracts / Serbian Ceramic Society Conference Advanced Ceramics and Application X New Frontiers in Multifunctional Material Science and Processing, Serbia, Belgrade, 26-27. September 2022.
Belgrade : Serbian Ceramic Society., 90-90.
https://hdl.handle.net/21.15107/rcub_dais_13627
Vujančević J, Blagojević VA, Andričević P, Pavlović VP, Horváth E, Forró L, Vlahović B, Pavlović VB, Janaćković Đ. Characteristic of photodiode based on vanadium oxide-TiO2 nanotubes/CH3NH3PbI3. in Program and the Book of abstracts / Serbian Ceramic Society Conference Advanced Ceramics and Application X New Frontiers in Multifunctional Material Science and Processing, Serbia, Belgrade, 26-27. September 2022.. 2022;:90-90.
https://hdl.handle.net/21.15107/rcub_dais_13627 .
Vujančević, Jelena, Blagojević, Vladimir A., Andričević, Pavao, Pavlović, Vera P., Horváth, Endre, Forró, László, Vlahović, Branislav, Pavlović, Vladimir B., Janaćković, Đorđe, "Characteristic of photodiode based on vanadium oxide-TiO2 nanotubes/CH3NH3PbI3" in Program and the Book of abstracts / Serbian Ceramic Society Conference Advanced Ceramics and Application X New Frontiers in Multifunctional Material Science and Processing, Serbia, Belgrade, 26-27. September 2022. (2022):90-90,
https://hdl.handle.net/21.15107/rcub_dais_13627 .

Influence of anodization voltage on photocatalztic activity of TiO2 nanotubes

Vujančević, Jelena; Ćirković, Jovana; Horváth, Endre; Forró, László; Pavlović, Vladimir B.; Janaćković, Đorđe

(Belgrade : Innovation Center of Faculty of Mechanical Engineering, 2021)

TY  - CONF
AU  - Vujančević, Jelena
AU  - Ćirković, Jovana
AU  - Horváth, Endre
AU  - Forró, László
AU  - Pavlović, Vladimir B.
AU  - Janaćković, Đorđe
PY  - 2021
UR  - https://dais.sanu.ac.rs/123456789/12347
AB  - TiO2 under UV light generates charge carriers (electrons and holes) that take part in the process of decomposition of pollutants, which is a well-known fact for the past few decades. For this reason, TiO2 is used for photocatalytic purification water and air. Photoactivity of TiO2 depends on the amount of generated charge carriers, and one part of those carriers are lost through the process of recombination. In order to improve photoactivity, it is necessary to speed up transport of electrons and holes. For better and faster charge carrier transport a unidirectional path is desired, which can be obtained by synthesizing 1D morphology. Anodization of titanium foil is a good way to obtain perpendicular nanotubular morphology onto a substrate. Nanotubular morphology can be optimized via operative conditions of anodization: applied voltage, anodization time and type of electrolyte. In this work, TiO2 nanotube arrays were synthesized by anodization of titanium foil at different voltages: 10 V, 15 V, 20 V and 25 V. Based on FESEM (Field Emission Scanning Electron Microscopy) micrographs, the microstructure of nanotubes was analysed and data concerning wall thickness, outer diameter of nanotubes and active surface were considered. Also, the influence of nanotube morphology on optical properties was determined. Results of our research show that the increasement in anodization voltage influenced on the appearance of redshift in the absorption spectrum. The sample synthesized at 20 V showed the highest photocatalytic activity due to the optimal nanotube length and nanotube diameter.
PB  - Belgrade : Innovation Center of Faculty of Mechanical Engineering
C3  - Programme and The Book of Abstracts / International Conference of Experimental and Numerical Investigations and New Technologies - CNN TECH 2021,29 June - 02 July 2021, Zlatibor, Serbia
T1  - Influence of anodization voltage on photocatalztic activity of TiO2 nanotubes
SP  - 23
EP  - 23
UR  - https://hdl.handle.net/21.15107/rcub_dais_12347
ER  - 
@conference{
author = "Vujančević, Jelena and Ćirković, Jovana and Horváth, Endre and Forró, László and Pavlović, Vladimir B. and Janaćković, Đorđe",
year = "2021",
abstract = "TiO2 under UV light generates charge carriers (electrons and holes) that take part in the process of decomposition of pollutants, which is a well-known fact for the past few decades. For this reason, TiO2 is used for photocatalytic purification water and air. Photoactivity of TiO2 depends on the amount of generated charge carriers, and one part of those carriers are lost through the process of recombination. In order to improve photoactivity, it is necessary to speed up transport of electrons and holes. For better and faster charge carrier transport a unidirectional path is desired, which can be obtained by synthesizing 1D morphology. Anodization of titanium foil is a good way to obtain perpendicular nanotubular morphology onto a substrate. Nanotubular morphology can be optimized via operative conditions of anodization: applied voltage, anodization time and type of electrolyte. In this work, TiO2 nanotube arrays were synthesized by anodization of titanium foil at different voltages: 10 V, 15 V, 20 V and 25 V. Based on FESEM (Field Emission Scanning Electron Microscopy) micrographs, the microstructure of nanotubes was analysed and data concerning wall thickness, outer diameter of nanotubes and active surface were considered. Also, the influence of nanotube morphology on optical properties was determined. Results of our research show that the increasement in anodization voltage influenced on the appearance of redshift in the absorption spectrum. The sample synthesized at 20 V showed the highest photocatalytic activity due to the optimal nanotube length and nanotube diameter.",
publisher = "Belgrade : Innovation Center of Faculty of Mechanical Engineering",
journal = "Programme and The Book of Abstracts / International Conference of Experimental and Numerical Investigations and New Technologies - CNN TECH 2021,29 June - 02 July 2021, Zlatibor, Serbia",
title = "Influence of anodization voltage on photocatalztic activity of TiO2 nanotubes",
pages = "23-23",
url = "https://hdl.handle.net/21.15107/rcub_dais_12347"
}
Vujančević, J., Ćirković, J., Horváth, E., Forró, L., Pavlović, V. B.,& Janaćković, Đ.. (2021). Influence of anodization voltage on photocatalztic activity of TiO2 nanotubes. in Programme and The Book of Abstracts / International Conference of Experimental and Numerical Investigations and New Technologies - CNN TECH 2021,29 June - 02 July 2021, Zlatibor, Serbia
Belgrade : Innovation Center of Faculty of Mechanical Engineering., 23-23.
https://hdl.handle.net/21.15107/rcub_dais_12347
Vujančević J, Ćirković J, Horváth E, Forró L, Pavlović VB, Janaćković Đ. Influence of anodization voltage on photocatalztic activity of TiO2 nanotubes. in Programme and The Book of Abstracts / International Conference of Experimental and Numerical Investigations and New Technologies - CNN TECH 2021,29 June - 02 July 2021, Zlatibor, Serbia. 2021;:23-23.
https://hdl.handle.net/21.15107/rcub_dais_12347 .
Vujančević, Jelena, Ćirković, Jovana, Horváth, Endre, Forró, László, Pavlović, Vladimir B., Janaćković, Đorđe, "Influence of anodization voltage on photocatalztic activity of TiO2 nanotubes" in Programme and The Book of Abstracts / International Conference of Experimental and Numerical Investigations and New Technologies - CNN TECH 2021,29 June - 02 July 2021, Zlatibor, Serbia (2021):23-23,
https://hdl.handle.net/21.15107/rcub_dais_12347 .

Photoactivity of vanadium oxide TiO2 nanotubes

Vujančević, Jelena; Blagojević, Vladimir; Andričević, Pavao; Pavlović, Vera P.; Horváth, Endre; Forró, László; Vlahović, Branislav; Pavlović, Vladimir B.; Janaćković, Đorđe

(Novi Sad : Faculty of Technology, 2021)

TY  - CONF
AU  - Vujančević, Jelena
AU  - Blagojević, Vladimir
AU  - Andričević, Pavao
AU  - Pavlović, Vera P.
AU  - Horváth, Endre
AU  - Forró, László
AU  - Vlahović, Branislav
AU  - Pavlović, Vladimir B.
AU  - Janaćković, Đorđe
PY  - 2021
UR  - https://dais.sanu.ac.rs/123456789/12398
AB  - The aim of this study was to investigate the influence of vanadium oxide photosensitive surface layer on the photoactivity of TiO2 nanotubes. Nanotube arrays were synthesized by anodization of titanium foil at different voltages, and vanadium-oxide was deposited by wet chemical deposition. Deposition of the vanadium-oxide layer was confirmed by XPS analysis, which provided the chemical composition of the sample surface. Photovoltaic characteristics and photocatalytic performance for photodegradation of methyl orange dye of modified TiO2 nanotubes were correlated with the nanotube morphology (and anodization voltage). Optimal anodization voltage was determined, in conjunction with the deposition of the surface vanadium oxide layer, in order to achieve maximum performance of the modified TiO2 electrodes. This has been correlated with changes in the optical properties of the TiO2 electrodes, the nanotube length and diameter, as they occur with the change in the anodization voltage, as well as the changes in the vanadium-oxide content in the samples, where the vanadium-oxide content was found to be determined by the nanotube morphology. The photovoltaic performance of the optimized modified TiO2 electrode with the surface vanadium-oxide layer was found to be significantly better than both the performance of the corresponding TiO2 electrode, and the performance of all the other TiO2 electrodes included in the study.
PB  - Novi Sad : Faculty of Technology
C3  - Programme and book of abstracts / 14th ECerS Conference for Young Scientists in Ceramics (CYSC-2021), October 20-23, 2021, Novi Sad
T1  - Photoactivity of vanadium oxide TiO2 nanotubes
SP  - 92
EP  - 92
UR  - https://hdl.handle.net/21.15107/rcub_dais_12398
ER  - 
@conference{
author = "Vujančević, Jelena and Blagojević, Vladimir and Andričević, Pavao and Pavlović, Vera P. and Horváth, Endre and Forró, László and Vlahović, Branislav and Pavlović, Vladimir B. and Janaćković, Đorđe",
year = "2021",
abstract = "The aim of this study was to investigate the influence of vanadium oxide photosensitive surface layer on the photoactivity of TiO2 nanotubes. Nanotube arrays were synthesized by anodization of titanium foil at different voltages, and vanadium-oxide was deposited by wet chemical deposition. Deposition of the vanadium-oxide layer was confirmed by XPS analysis, which provided the chemical composition of the sample surface. Photovoltaic characteristics and photocatalytic performance for photodegradation of methyl orange dye of modified TiO2 nanotubes were correlated with the nanotube morphology (and anodization voltage). Optimal anodization voltage was determined, in conjunction with the deposition of the surface vanadium oxide layer, in order to achieve maximum performance of the modified TiO2 electrodes. This has been correlated with changes in the optical properties of the TiO2 electrodes, the nanotube length and diameter, as they occur with the change in the anodization voltage, as well as the changes in the vanadium-oxide content in the samples, where the vanadium-oxide content was found to be determined by the nanotube morphology. The photovoltaic performance of the optimized modified TiO2 electrode with the surface vanadium-oxide layer was found to be significantly better than both the performance of the corresponding TiO2 electrode, and the performance of all the other TiO2 electrodes included in the study.",
publisher = "Novi Sad : Faculty of Technology",
journal = "Programme and book of abstracts / 14th ECerS Conference for Young Scientists in Ceramics (CYSC-2021), October 20-23, 2021, Novi Sad",
title = "Photoactivity of vanadium oxide TiO2 nanotubes",
pages = "92-92",
url = "https://hdl.handle.net/21.15107/rcub_dais_12398"
}
Vujančević, J., Blagojević, V., Andričević, P., Pavlović, V. P., Horváth, E., Forró, L., Vlahović, B., Pavlović, V. B.,& Janaćković, Đ.. (2021). Photoactivity of vanadium oxide TiO2 nanotubes. in Programme and book of abstracts / 14th ECerS Conference for Young Scientists in Ceramics (CYSC-2021), October 20-23, 2021, Novi Sad
Novi Sad : Faculty of Technology., 92-92.
https://hdl.handle.net/21.15107/rcub_dais_12398
Vujančević J, Blagojević V, Andričević P, Pavlović VP, Horváth E, Forró L, Vlahović B, Pavlović VB, Janaćković Đ. Photoactivity of vanadium oxide TiO2 nanotubes. in Programme and book of abstracts / 14th ECerS Conference for Young Scientists in Ceramics (CYSC-2021), October 20-23, 2021, Novi Sad. 2021;:92-92.
https://hdl.handle.net/21.15107/rcub_dais_12398 .
Vujančević, Jelena, Blagojević, Vladimir, Andričević, Pavao, Pavlović, Vera P., Horváth, Endre, Forró, László, Vlahović, Branislav, Pavlović, Vladimir B., Janaćković, Đorđe, "Photoactivity of vanadium oxide TiO2 nanotubes" in Programme and book of abstracts / 14th ECerS Conference for Young Scientists in Ceramics (CYSC-2021), October 20-23, 2021, Novi Sad (2021):92-92,
https://hdl.handle.net/21.15107/rcub_dais_12398 .