Dielectric Properties of Mechanically Activated Strontium Titanate Ceramics
Autori
Živojinović, JelenaKosanović, Darko
Blagojević, Vladimir A.
Pavlović, Vera P.
Tadić, Nenad
Vlahović, Branislav
Pavlović, Vladimir B.
Članak u časopisu (Objavljena verzija)
Metapodaci
Prikaz svih podataka o dokumentuApstrakt
In this study, microstructure evolution and dielectric properties of SrTiO3 ceramic have been investigated, whereby mechanical activation of SrTiO3 powders was used to modify the functional properties of ceramic materials. Microstructural SEM analysis of SrTiO3 ceramics showed that the increase in mechanical activation time results in less porous samples. Raman spectroscopy indicated changes in the broadening and asymmetry of the TO2 mode with a change in the time of mechanical activation. TO2 mode showed a Fano asymmetry due to its interaction with polarization fluctuations in polar micro-regions, which are a consequence of the presence of oxygen vacancies caused by activation. The maximum value of dielectric permittivity was observed in the sample activated for 10 min. Also, the sample activated for 10 min exhibits relatively low values of loss tangent, compared to the other mechanically activated samples, providing the best overall dielectric performance compared to other samples.
Izvor:
Science of Sintering, 2022, 54, 4, 401-414Finansiranje / projekti:
- Ministarstvo nauke, tehnološkog razvoja i inovacija Republike Srbije, institucionalno finansiranje - 200175 (Institut tehničkih nauka SANU, Beograd) (RS-MESTD-inst-2020-200175)
- Ministarstvo nauke, tehnološkog razvoja i inovacija Republike Srbije, institucionalno finansiranje - 200105 (Univerzitet u Beogradu, Mašinski fakultet) (RS-MESTD-inst-2020-200105)
- Ministarstvo nauke, tehnološkog razvoja i inovacija Republike Srbije, institucionalno finansiranje - 200116 (Univerzitet u Beogradu, Poljoprivredni fakultet) (RS-MESTD-inst-2020-200116)
- National Science Foundation grant HRD-1345219
- National Science Foundation grant DMR-1523617
Institucija/grupa
Институт техничких наука САНУ / Institute of Technical Sciences of SASATY - JOUR AU - Živojinović, Jelena AU - Kosanović, Darko AU - Blagojević, Vladimir A. AU - Pavlović, Vera P. AU - Tadić, Nenad AU - Vlahović, Branislav AU - Pavlović, Vladimir B. PY - 2022 UR - https://dais.sanu.ac.rs/123456789/13510 AB - In this study, microstructure evolution and dielectric properties of SrTiO3 ceramic have been investigated, whereby mechanical activation of SrTiO3 powders was used to modify the functional properties of ceramic materials. Microstructural SEM analysis of SrTiO3 ceramics showed that the increase in mechanical activation time results in less porous samples. Raman spectroscopy indicated changes in the broadening and asymmetry of the TO2 mode with a change in the time of mechanical activation. TO2 mode showed a Fano asymmetry due to its interaction with polarization fluctuations in polar micro-regions, which are a consequence of the presence of oxygen vacancies caused by activation. The maximum value of dielectric permittivity was observed in the sample activated for 10 min. Also, the sample activated for 10 min exhibits relatively low values of loss tangent, compared to the other mechanically activated samples, providing the best overall dielectric performance compared to other samples. T2 - Science of Sintering T1 - Dielectric Properties of Mechanically Activated Strontium Titanate Ceramics SP - 401 EP - 414 VL - 54 IS - 4 DO - 10.2298/SOS2204401Z UR - https://hdl.handle.net/21.15107/rcub_dais_13510 ER -
@article{ author = "Živojinović, Jelena and Kosanović, Darko and Blagojević, Vladimir A. and Pavlović, Vera P. and Tadić, Nenad and Vlahović, Branislav and Pavlović, Vladimir B.", year = "2022", abstract = "In this study, microstructure evolution and dielectric properties of SrTiO3 ceramic have been investigated, whereby mechanical activation of SrTiO3 powders was used to modify the functional properties of ceramic materials. Microstructural SEM analysis of SrTiO3 ceramics showed that the increase in mechanical activation time results in less porous samples. Raman spectroscopy indicated changes in the broadening and asymmetry of the TO2 mode with a change in the time of mechanical activation. TO2 mode showed a Fano asymmetry due to its interaction with polarization fluctuations in polar micro-regions, which are a consequence of the presence of oxygen vacancies caused by activation. The maximum value of dielectric permittivity was observed in the sample activated for 10 min. Also, the sample activated for 10 min exhibits relatively low values of loss tangent, compared to the other mechanically activated samples, providing the best overall dielectric performance compared to other samples.", journal = "Science of Sintering", title = "Dielectric Properties of Mechanically Activated Strontium Titanate Ceramics", pages = "401-414", volume = "54", number = "4", doi = "10.2298/SOS2204401Z", url = "https://hdl.handle.net/21.15107/rcub_dais_13510" }
Živojinović, J., Kosanović, D., Blagojević, V. A., Pavlović, V. P., Tadić, N., Vlahović, B.,& Pavlović, V. B.. (2022). Dielectric Properties of Mechanically Activated Strontium Titanate Ceramics. in Science of Sintering, 54(4), 401-414. https://doi.org/10.2298/SOS2204401Z https://hdl.handle.net/21.15107/rcub_dais_13510
Živojinović J, Kosanović D, Blagojević VA, Pavlović VP, Tadić N, Vlahović B, Pavlović VB. Dielectric Properties of Mechanically Activated Strontium Titanate Ceramics. in Science of Sintering. 2022;54(4):401-414. doi:10.2298/SOS2204401Z https://hdl.handle.net/21.15107/rcub_dais_13510 .
Živojinović, Jelena, Kosanović, Darko, Blagojević, Vladimir A., Pavlović, Vera P., Tadić, Nenad, Vlahović, Branislav, Pavlović, Vladimir B., "Dielectric Properties of Mechanically Activated Strontium Titanate Ceramics" in Science of Sintering, 54, no. 4 (2022):401-414, https://doi.org/10.2298/SOS2204401Z ., https://hdl.handle.net/21.15107/rcub_dais_13510 .